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    $\begingroup$ The selected edge in the lower image is no loop edge. See this answer: Alt+Left Click doesn't select Loops on sharp edges (<90°) $\endgroup$ Commented Mar 28, 2023 at 10:46
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    $\begingroup$ If you want to select the edges around a face, select the face in Face mode (3 on the keyboard) and then change to Edge mode (2). $\endgroup$
    – John Eason
    Commented Mar 28, 2023 at 11:02
  • $\begingroup$ The perimeter of the face is not a valid loop.. is that the one you're hoping for? so. which face? $\endgroup$
    – Robin Betts
    Commented Mar 28, 2023 at 18:21