It is possible to do this. There are 3 parts to LVM -
- The Physical Volume
- The Volume Group
- Logical Volumes
So the way I would do this is to create a partition on the second disk (you don't need to do this, but its the "correct" way to do it)
First instruct the Operating system that you have 2 Physical Volumes you wish to assign to LVM - you do this by running the following command for each of the 2 partitions
pvcreate /dev/sdXX
The second step is to assign both physical volumes into 1 volume group -
vgcreate vgname /dev/sdXX /dev/sdXX
The third step is to create a logical volume
lvcreate -n NewPartitionName vg -L 899G
In this example I've created an 899 gig block device which will be called /dev/vgname/NewPartitionName. Depending on your needs, seriously consider starting off only using, say 800 Gigs of space, leaving the last 99 gigs free - this will give you freedom to create additional volumes - including snapshots, which can be useful. You can always expand the current volume later (even when the filesystem is in use). Its is easier to make a volume bigger then smaller.
At this stage you are ready to add your filesystem. Not sure if you need help here, but you could use a command mkfs.ext4 /dev/vgname/NewPartitionName to format the partition. You can then add it to your fstab file if you want it to be automatically mounted.